December 2021

Wave-particle duality and entanglement are two fundamental characteristics of quantum mechanics. All previous works on experimental investigations in wave{particle properties of single photons (or single particles in general) show that a well-defined interferometer setting determines a well-defined property of single photons. Here we take a conceptual step forward and control the wave-particle property of single photons with quantum entanglement. By doing so, we experimentally test the complementarity principle in a scenario, in which the setting of the interferometer is not defined at any instance of the experiment, not even in principle. To achieve this goal, we send the photon of interest (S) into a quantum Mach-Zehnder interferometer (MZI), in which the output beam splitter of the MZI is controlled by the quantum state of the second photon (C), who is entangled with a third photon (A). Therefore, the individual quantum state of photon C is undefined, which implements the undefined settings of the MZI for photon S. This is realized by using three cascaded phase-stable interferometers for three photons. There is typically no well-defined setting of the MZI, and thus the very formulation of the wave-particle properties becomes internally inconsistent.

In the quantization of gauge theories and quantum gravity, it is crucial to treat reference frames such as rods or clocks not as idealized external classical relata, but as internal quantum subsystems. In the Page-Wootters formalism, for example, evolution of a quantum system S is described by a stationary joint state of S and a quantum clock, where time-dependence of S arises from conditioning on the value of the clock. Here, we consider (possibly imperfect) internal quantum reference frames R for arbitrary compact symmetry groups, and show that there is an exact quantitative correspondence between the amount of entanglement in the invariant state on RS and the amount of asymmetry in the corresponding conditional state on S. Surprisingly, this duality holds exactly regardless of the choice of coherent state system used to condition on the reference frame. Averaging asymmetry over all conditional states, we obtain a simple representation-theoretic expression that admits the study of the quality of imperfect quantum reference frames, quantum speed limits for imperfect clocks, and typicality of asymmetry in a unified way. Our results shed light on the role of entanglement for establishing asymmetry in a fully symmetric quantum world.